Cavity ringdown laser absorption spectroscopy and time‐of‐flight mass spectroscopy of jet cooled platinum silicides

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Cavity ringdown laser absorption spectroscopy and time-of-flight mass spectroscopy of jet cooled platinum silicides.

The cavity ringdown technique (CRLAS) has been employed to measure the gas phase absorption spectrum of the platinum silicide molecule in the 350 nm region. All nine of the measured rovibronic bands are assigned to a single 1 sigma-1 sigma electronic transition, with a ground state vibrational frequency of omega "e = 549.0(3) cm-1, and a bond length of r"0 = 2.069(1) angstroms. The results of...

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Cavity ringdown laser absorption spectroscopy and time-of-flight mass spectroscopy of jet-cooled gold silicides

The cavity ringdown technique has been employed for the spectroscopic characterization of the AuSi molecule, which is generated in a pulsed supersonic laser vaporization plasma reactor. Fifteen rovibronic bands have been measured between 340 nm–390 nm, 8 of which have been analyzed to yield molecular properties for the X and D S states of AuSi. This assignment is in disagreement with previous e...

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Cavity ringdown laser absorption spectroscopy and time-of-flight mass spectroscopy of jet-cooled silver silicides

The cavity ringdown technique has been employed for the first spectroscopic characterization of the AgSi molecule, which is generated in a pulsed laser vaporization plasma reactor. A total of 20 rovibronic bands between 365 and 385 nm have been measured and analyzed to yield molecular properties for the X , B , and C S states of AgSi. A time-of-flight mass spectrometer simultaneously monitors s...

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Cavity ringdown laser absorption spectroscopy and time-of-flight mass spectroscopy of jet-cooled copper silicides

The cavity ringdown technique has been implemented for electronic spectroscopy of jet-cooled CuSi produced in a pulsed UV laser vaporization plasma reactor. A time-of-flight mass spectrometer is used to simultaneously monitor species produced in the supersonic expansion and allows correlation studies to be performed. Seven rotationally resolved vibronic bands have been measured near 400 nm, yie...

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Infrared cavity ringdown spectroscopy of jet-cooled polycyclic aromatic hydrocarbons.

Infrared absorption spectra of the CH stretching region were observed for naphthalene, anthracene, phenanthrene, pyrene, and perylene using a heated, supersonic, slit-jet source and cavity ringdown spectroscopy. Band positions and intensities recorded with 0.2-cm-1 resolution were compared with previous gas-phase and argon matrix isolation experiments, as well as theoretical calculations. The l...

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ژورنال

عنوان ژورنال: The Journal of Chemical Physics

سال: 1996

ISSN: 0021-9606,1089-7690

DOI: 10.1063/1.471101